Strange-metal behavior without fine tuning in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>PrV</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi>Al</mml:mi><mml:mn>20</mml:mn></mml:msub></mml:mrow></mml:ma

Strange-metal behavior observed in the praseodymium-based heavy-fermion material <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mrow><a:msub><a:mi>PrV</a:mi><a:mn>2</a:mn></a:msub><a:msub><a:mi>Al</a:mi><a:mn>20</a:mn></a:msub></a:mrow></a:math> has been tentatively interpreted in the framework of proximity to a quantum critical point (QCP) associated with quadrupolar ordering. Here, we demonstrate that an alternative, natural explanation exists without invoking a QCP, in terms of the unconventional nature of the quadrupolar Kondo effect taking place in non-Kramers ions. Using a combination of density-functional theory calculations and analytical arguments, we construct a periodic Anderson model with realistic parameters to describe <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:mrow><b:msub><b:mi>PrV</b:mi><b:mn>2</b:mn></b:msub><b:msub><b:mi>Al</b:mi><b:mn>20</b:mn></b:msub></b:mrow></b:math>. We solve the model using dynamical mean-field theory preserving the model symmetries and demonstrate the non-Fermi liquid strange-metal behavior stemming from the two-channel nature of the quadrupolar Kondo effect. Our calculations provide an explanation for the puzzling temperature dependence in the magnetic susceptibility and provide a basis for analyzing future photoemission experiments. Published by the American Physical Society 2024

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Publication Details

Journal
Physical Review Research
Published
2024-10-08
DOI
https://doi.org/10.1103/physrevresearch.6.l042008
Citations
1
Primary Topic
Rare-earth and actinide compounds
Type
article
Field-Weighted Citation Impact
0.31

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article

Strange-metal behavior without fine tuning in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>PrV</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi>Al</mml:mi><mml:mn>20</mml:mn></mml:msub></mml:mrow></mml:ma

Marvin Lenk, Andriy H. Nevidomskyy, Johann Kroha, Fei Gao
1 citations
Physical Review Research
Rare-earth and actinide compounds
0.31
article

Strange-metal behavior without fine tuning in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>PrV</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi>Al</mml:mi><mml:mn>20</mml:mn></mml:msub></mml:mrow></mml:ma

Marvin Lenk, Andriy H. Nevidomskyy, Johann Kroha, Fei Gao
article en
1 citations

Abstract

Strange-metal behavior observed in the praseodymium-based heavy-fermion material <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mrow><a:msub><a:mi>PrV</a:mi><a:mn>2</a:mn></a:msub><a:msub><a:mi>Al</a:mi><a:mn>20</a:mn></a:msub></a:mrow></a:math> has been tentatively interpreted in the framework of proximity to a quantum critical point (QCP) associated with quadrupolar ordering. Here, we demonstrate that an alternative, natural explanation exists without invoking a QCP, in terms of the unconventional nature of the quadrupolar Kondo effect taking place in non-Kramers ions. Using a combination of density-functional theory calculations and analytical arguments, we construct a periodic Anderson model with realistic parameters to describe <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:mrow><b:msub><b:mi>PrV</b:mi><b:mn>2</b:mn></b:msub><b:msub><b:mi>Al</b:mi><b:mn>20</b:mn></b:msub></b:mrow></b:math>. We solve the model using dynamical mean-field theory preserving the model symmetries and demonstrate the non-Fermi liquid strange-metal behavior stemming from the two-channel nature of the quadrupolar Kondo effect. Our calculations provide an explanation for the puzzling temperature dependence in the magnetic susceptibility and provide a basis for analyzing future photoemission experiments. Published by the American Physical Society 2024

Physical Review ResearchVol. 6(4)
University of Bonn (DE), University of St Andrews (GB), Rice University (US)
National Science Foundation, Aspen Center for Physics, Rice University, Deutsche Forschungsgemeinschaft, Rheinische Friedrich-Wilhelms-Universität Bonn, Division of Materials Research
Openalex Percentile: Top 43%
Rare-earth and actinide compounds
0.31
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