Probing Mie-resonant nanoparticles with swift electron beams

We discuss the richness of information that one can extract about the optical response of Mie-resonant high-index dielectric nanoparticles, when excited by a swift electron beam, in electron-energy loss or cathodoluminescence spectroscopy measurements. In particular, we analyse how, apart from Mie modes of electric or magnetic multipolar type, electron beams passing nearby or through the particle can produce a diversity of resonant or interference spectral features, due to the interaction of Mie modes with transition or Cherenkov radiation, or with intrinsic material processes such as interband transitions. We thus highlight the importance of precise analytic or semi-analytic theoretical approaches for the interpretation of measured or simulated spectra.

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Published
2024-09-09
DOI
https://doi.org/10.1109/metamaterials62190.2024.10703273
Primary Topic
Quantum Dots Synthesis And Properties
Type
article
Field-Weighted Citation Impact
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article

Probing Mie-resonant nanoparticles with swift electron beams

P. Elli Stamatopoulou, N. Asger Mortensen, Christos Tserkezis, Christian Wolff
Quantum Dots Synthesis And Properties
article

Probing Mie-resonant nanoparticles with swift electron beams

P. Elli Stamatopoulou, N. Asger Mortensen, Christos Tserkezis, Christian Wolff
article en

Abstract

We discuss the richness of information that one can extract about the optical response of Mie-resonant high-index dielectric nanoparticles, when excited by a swift electron beam, in electron-energy loss or cathodoluminescence spectroscopy measurements. In particular, we analyse how, apart from Mie modes of electric or magnetic multipolar type, electron beams passing nearby or through the particle can produce a diversity of resonant or interference spectral features, due to the interaction of Mie modes with transition or Cherenkov radiation, or with intrinsic material processes such as interband transitions. We thus highlight the importance of precise analytic or semi-analytic theoretical approaches for the interpretation of measured or simulated spectra.

University of Southern Denmark (DK)
National Research Foundation
Affordable and clean energy
Openalex Percentile: Top 89%
Quantum Dots Synthesis And Properties
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Probing Mie-resonant nanoparticles with swift electron beams — P. Elli Stamatopoulou, N. Asger Mortensen, et al. · (2024) | TGRS Research Map | TGRS