A Framework to Identify Supercritical and Subcritical Turing Bifurcations: Case Study of Soai Reaction Featuring Asymmetric Autocatalysis
In this work, we focus on an autocatalytic reaction–diffusion model and carry out multiple-scale weakly nonlinear analysis. A cubic and a quadratic autocatalytic reaction system is analyzed. We develop a framework to identify the critical surfaces in parameter space across which the nature of the Turing bifurcation changes from supercritical to subcritical. These are verified by numerical simulations of the system using Chebyshev spectral collocation method. Using weakly nonlinear analysis, we derive the amplitude equations up to the fifth order. This helps determine accurately the limit point of the bifurcating solution. The numerical solutions are in good agreement with the predictions of the weakly nonlinear analysis for supercritical bifurcations. We show that when multiple steady states arise, Turing patterns can coexist with other spatially uniform steady states. Furthermore, we show that our framework can be extended to get different patterns, such as squares, in a two-dimensional domain. This study will help identify operating conditions where Turing patterns can be obtained for reaction–diffusion systems.
Authors
- Deepak Kumar (ORCID: https://orcid.org/0009-0005-9174-2636)
- S. Pushpavanam (ORCID: https://orcid.org/0000-0002-5782-0670)
- Uttam Kumar (ORCID: https://orcid.org/0000-0002-0751-9388)
Institutions
- Indian Institute of Technology Madras (IN)
Publication Details
- Journal
- The Journal of Physical Chemistry C
- Published
- 2024-10-07
- DOI
- https://doi.org/10.1021/acs.jpcc.4c05116
- Primary Topic
- Nonlinear Dynamics and Pattern Formation
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Indian Institute of Technology Madras