Enhancement of photoresponse for InGaAs infrared photodetectors using plasmonic WO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mrow> <mml:mn>3</mml:mn> <mml:mo>−</mml:mo> <mml:mi>x</mml:mi> </mml:m

Fast and accurate detection of light in the near-infrared (NIR) spectral range plays a crucial role in modern society, from alleviating speed and capacity bottlenecks in optical communications to enhancing the control and safety of autonomous vehicles through NIR imaging systems. Several technological platforms are currently under investigation to improve NIR photodetection, aiming to surpass the performance of established III-V semiconductor p-i-n (PIN) junction technology. These platforms include<i>in situ</i>-grown inorganic nanocrystals (NCs) and nanowire arrays, as well as hybrid organic-inorganic materials such as graphene-perovskite heterostructures. However, challenges remain in NC and nanowire growth, large-area fabrication of high-quality 2D materials, and the fabrication of devices for practical applications. Here, we explore the potential for tailored semiconductor NCs to enhance the responsivity of planar metal-semiconductor-metal (MSM) photodetectors. MSM technology offers ease of fabrication and fast response times compared to PIN detectors. We observe enhancement of the optical-to-electric conversion efficiency by up to a factor of ∼2.5 through the application of plasmonically-active semiconductor nanorods and NCs. We present a protocol for synthesizing and rapidly testing the performance of non-stoichiometric tungsten oxide (WO3-x) nanorods and cesium-doped tungsten oxide (Cs<sub><i>y</i></sub>WO3-x) hexagonal nanoprisms prepared in colloidal suspensions and drop-cast onto photodetector surfaces. The results demonstrate the potential for a cost-effective and scalable method exploiting tailored NCs to improve the performance of NIR optoelectronic devices.

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Publication Details

Journal
Nanotechnology
Published
2024-10-03
DOI
https://doi.org/10.1088/1361-6528/ad82f1
Citations
2
Primary Topic
Ga2O3 and related materials
Type
article
Field-Weighted Citation Impact
0.24

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article

Enhancement of photoresponse for InGaAs infrared photodetectors using plasmonic WO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mrow> <mml:mn>3</mml:mn> <mml:mo>−</mml:mo> <mml:mi>x</mml:mi> </mml:m

Arjun Shetty, Jonathan Baugh, Man Chun Tam, Z. R. Wasilewski et al.
2 citations
Nanotechnology
Ga2O3 and related materials
0.24
article

Enhancement of photoresponse for InGaAs infrared photodetectors using plasmonic WO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mrow> <mml:mn>3</mml:mn> <mml:mo>−</mml:mo> <mml:mi>x</mml:mi> </mml:m

Arjun Shetty, Jonathan Baugh, Man Chun Tam, Z. R. Wasilewski, Zach D. Merino, Penghui Yin, Gyorgy Jaics, Pavle V. Radovanovic, Xinning Wang, Andrew W. M. Jordan
article en
2 citations

Abstract

Fast and accurate detection of light in the near-infrared (NIR) spectral range plays a crucial role in modern society, from alleviating speed and capacity bottlenecks in optical communications to enhancing the control and safety of autonomous vehicles through NIR imaging systems. Several technological platforms are currently under investigation to improve NIR photodetection, aiming to surpass the performance of established III-V semiconductor p-i-n (PIN) junction technology. These platforms include<i>in situ</i>-grown inorganic nanocrystals (NCs) and nanowire arrays, as well as hybrid organic-inorganic materials such as graphene-perovskite heterostructures. However, challenges remain in NC and nanowire growth, large-area fabrication of high-quality 2D materials, and the fabrication of devices for practical applications. Here, we explore the potential for tailored semiconductor NCs to enhance the responsivity of planar metal-semiconductor-metal (MSM) photodetectors. MSM technology offers ease of fabrication and fast response times compared to PIN detectors. We observe enhancement of the optical-to-electric conversion efficiency by up to a factor of ∼2.5 through the application of plasmonically-active semiconductor nanorods and NCs. We present a protocol for synthesizing and rapidly testing the performance of non-stoichiometric tungsten oxide (WO3-x) nanorods and cesium-doped tungsten oxide (Cs<sub><i>y</i></sub>WO3-x) hexagonal nanoprisms prepared in colloidal suspensions and drop-cast onto photodetector surfaces. The results demonstrate the potential for a cost-effective and scalable method exploiting tailored NCs to improve the performance of NIR optoelectronic devices.

NanotechnologyVol. 36(1)
University of Waterloo (CA)
Canada Foundation for Innovation, Canada First Research Excellence Fund, Natural Sciences and Engineering Research Council of Canada
Openalex Percentile: Top 58%
Ga2O3 and related materials
0.24
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