Surface Chemical Effects on Fischer–Tropsch Iron Oxide Catalysts Caused by Alkali Ion (Li, Na, K, Cs) Doping
Among the alkali metals, potassium is known to significantly shift selectivity toward value-added, heavier alkanes and olefins in iron-based Fischer–Tropsch synthesis catalysts. The aim of the present contribution is to shed light on the mechanism of action of alkaline promoters through a systematic study of the structure–reactivity relationships of a series of Fe oxide FTS catalysts promoted with Group I (Li, Na, K, Cs) alkali elements. Reactivity data are compared to structural data based on in situ, synchrotron-based XRD and XPS, as well as temperature-programmed studies (TPR-H2, TPC-CO, TPD-CO2, and TPD-H). It has been observed that the alkali elements induced higher carburization rates, higher basicities, and lower adsorbed hydrogen coverages. Catalyst stability followed the trend Na-Fe > unpromoted > Li-Fe > K-Fe > Cs-Fe, being consistent with the ability of the alkali (Na) to prevent active site loss by catalyst reoxidation. Potassium was the most active in promoting high α hydrocarbon formation. It is active enough to promote CO dissociative adsorption (and the formation of FeCx active phases) and decrease the surface coverage of H-adsorbed species, but it is not so active as to cause premature catalyst deactivation by the formation of a carbon layer resulting in the blocking active sites.
Authors
- Mauro C. Ribeiro
- Igor Ferreira Gomes
- Jóice Cleide Cardoso Ennes de Souza (ORCID: https://orcid.org/0000-0002-3848-4923)
- Mirtha Z. Leguizamón León Ribeiro
- Gary Jacobs (ORCID: https://orcid.org/0000-0003-0691-6717)
- Muthu Kumaran Gnanamani (ORCID: https://orcid.org/0000-0003-1274-2645)
- Michela Martinelli (ORCID: https://orcid.org/0000-0003-1231-6419)
Institutions
- University of Kentucky (US)
- Universidade Federal Fluminense (BR)
- The University of Texas at San Antonio (US)
- Universidad Nacional de Asunción (PY)
Publication Details
- Journal
- Catalysts
- Published
- 2024-10-02
- DOI
- https://doi.org/10.3390/catal14100682
- Citations
- 5
- Primary Topic
- Catalysts for Methane Reforming
- Type
- article
- Field-Weighted Citation Impact
- 0.53
Funders
- Ministério da Ciência, Tecnologia e Inovação
- Centro Nacional de Pesquisa em Energia e Materiais
- Laboratório Nacional de Luz Síncrotron