Quantum Rectification Based on Room Temperature Multidirectional Nonlinearity in Bi<sub>2</sub>Te<sub>3</sub>

Recent interest in quantum nonlinearity has spurred the development of rectifiers for harvesting energy from ambient radiofrequency waves. However, these rectifiers face efficiency and bandwidth limitations at room temperature. We address these challenges by exploring Bi<sub>2</sub>Te<sub>3</sub>, a time-reversal symmetric topological quantum material. Bi<sub>2</sub>Te<sub>3</sub> exhibits robust room temperature second-order voltage generation in both the longitudinal and transverse directions. We harness these coexisting nonlinearities to design a multidirectional quantum rectifier that can simultaneously extract energy from various components of an input signal. We demonstrate the efficacy of Bi<sub>2</sub>Te<sub>3</sub>-based rectifiers across a broad frequency range, spanning from existing Wi-Fi bands (2.45 GHz) to frequencies relevant to next-generation 5G technology (27.4 GHz). Our Bi<sub>2</sub>Te<sub>3</sub>-based rectifier surpasses previous limitations by achieving a high rectification efficiency and operational frequency, alongside a low operational threshold and broadband functionality. These findings enable practical topological quantum rectifiers for high-frequency electronics and energy conversion, advancing wireless energy harvesting for next-generation communication.

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Publication Details

Journal
Nano Letters
Published
2024-09-27
DOI
https://doi.org/10.1021/acs.nanolett.4c03517
Citations
7
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
2.36

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Quantum Rectification Based on Room Temperature Multidirectional Nonlinearity in Bi2Te3

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article

Quantum Rectification Based on Room Temperature Multidirectional Nonlinearity in Bi2Te3

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article en
7 citations

Abstract

Recent interest in quantum nonlinearity has spurred the development of rectifiers for harvesting energy from ambient radiofrequency waves. However, these rectifiers face efficiency and bandwidth limitations at room temperature. We address these challenges by exploring Bi<sub>2</sub>Te<sub>3</sub>, a time-reversal symmetric topological quantum material. Bi<sub>2</sub>Te<sub>3</sub> exhibits robust room temperature second-order voltage generation in both the longitudinal and transverse directions. We harness these coexisting nonlinearities to design a multidirectional quantum rectifier that can simultaneously extract energy from various components of an input signal. We demonstrate the efficacy of Bi<sub>2</sub>Te<sub>3</sub>-based rectifiers across a broad frequency range, spanning from existing Wi-Fi bands (2.45 GHz) to frequencies relevant to next-generation 5G technology (27.4 GHz). Our Bi<sub>2</sub>Te<sub>3</sub>-based rectifier surpasses previous limitations by achieving a high rectification efficiency and operational frequency, alongside a low operational threshold and broadband functionality. These findings enable practical topological quantum rectifiers for high-frequency electronics and energy conversion, advancing wireless energy harvesting for next-generation communication.

Nano LettersVol. 24(40)
Indian Institute of Technology Ropar (IN), National University of Singapore (SG), Netaji Subhas University of Technology (IN)
Inspire Foundation, Agency for Science, Technology and Research, National Research Foundation Singapore
Climate action
Openalex Percentile: Top 11%
Topological Materials and Phenomena
2.36
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