Fast Fourier transform spectroscopy with broadband strongly modulated quantum cascade lasers

The combination of speed and resolution is a fundamental figure of merit for Fourier transform spectroscopy. Here, we show that, by combining a fast rotational delay line with a strongly modulated quantum cascade laser (QCL), it is possible to perform broadband spectroscopy over a range of 175 cm−1, with a total effective integration time of about 6 s and a resolution of 0.03 cm−1. Remarkably, even though the resolution of the measurement is limited by the source, the interleaving technique can still be applied when the QCL is not in a frequency comb regime, considerably broadening the bandwidth of the instrument.

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Publication Details

Journal
Applied Physics Letters
Published
2024-09-23
DOI
https://doi.org/10.1063/5.0226044
Citations
2
Primary Topic
Spectroscopy and Laser Applications
Type
article
Field-Weighted Citation Impact
0.48

Funders

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article

Fast Fourier transform spectroscopy with broadband strongly modulated quantum cascade lasers

Giacomo Scalari, Mathieu Bertrand, Jérôme Faist, Diego Piciocchi et al.
2 citations
Applied Physics Letters
Spectroscopy and Laser Applications
0.48
article

Fast Fourier transform spectroscopy with broadband strongly modulated quantum cascade lasers

Giacomo Scalari, Mathieu Bertrand, Jérôme Faist, Diego Piciocchi, Alessio Cargioli
article en
2 citations

Abstract

The combination of speed and resolution is a fundamental figure of merit for Fourier transform spectroscopy. Here, we show that, by combining a fast rotational delay line with a strongly modulated quantum cascade laser (QCL), it is possible to perform broadband spectroscopy over a range of 175 cm−1, with a total effective integration time of about 6 s and a resolution of 0.03 cm−1. Remarkably, even though the resolution of the measurement is limited by the source, the interleaving technique can still be applied when the QCL is not in a frequency comb regime, considerably broadening the bandwidth of the instrument.

Applied Physics LettersVol. 125(13)
ETH Zurich (CH)
Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung, Staatssekretariat für Bildung, Forschung und Innovation, National Center of Competence in Research Quantum Science and Technology
Affordable and clean energy
Openalex Percentile: Top 40%
Spectroscopy and Laser Applications
0.48
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Fast Fourier transform spectroscopy with broadband strongly modulated quantum cascade lasers — Giacomo Scalari, Mathieu Bertrand, et al. · Applied Physics Letters (2024) | TGRS Research Map | TGRS