High-Performance Red Transparent Quantum Dot Light-Emitting Diodes via Fully Solution-Processed MXene/Ag NWs Top Electrode

The integration of high-performance transparent top electrodes with the functional layers of transparent quantum dot light-emitting diodes (T-QLEDs) poses a notable challenge. This study presents a composite transparent top electrode composed of MXene and Ag NWs. The composite electrode demonstrates exceptional transparency (84.6% at 620 nm) and low sheet resistance (16.07 Ω sq<sup>-1</sup>), rendering it suitable for integration into T-QLEDs. The inclusion of MXene nanosheets in the composite electrode serves a dual role: adjusting the work function to enhance electron injection efficiency and enhancing the interface between Ag NWs and the emissive layer, thereby mitigating the common issue of interfacial resistance in conventional transparent electrodes. This strategic amalgamation results in notable improvements in device performance, yielding a maximum current efficiency of 23.12 cd A<sup>-1</sup>, an external quantum efficiency of 13.98%, and a brightness of 21,015 cd m<sup>-2</sup>. These performance metrics surpass those achieved by T-LEDs employing pristine Ag NW electrodes. This study offers valuable insights into T-QLED device advancement and provides a promising approach for transparent electrode fabrication in optoelectronic applications.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2024-09-26
DOI
https://doi.org/10.1021/acsami.4c11431
Citations
8
Primary Topic
Quantum Dots Synthesis And Properties
Type
article
Field-Weighted Citation Impact
0.94

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article

High-Performance Red Transparent Quantum Dot Light-Emitting Diodes via Fully Solution-Processed MXene/Ag NWs Top Electrode

Daojian Su, Peili Gao, Fanyuan Meng, Shuangpeng Wang et al.
8 citations
ACS Applied Materials & Interfaces
Quantum Dots Synthesis And Properties
0.94
article

High-Performance Red Transparent Quantum Dot Light-Emitting Diodes via Fully Solution-Processed MXene/Ag NWs Top Electrode

Daojian Su, Peili Gao, Fanyuan Meng, Shuangpeng Wang, Guoqiang Yuan, Yin‐Man Song, Xin He, Ting Ding, Hang Liu
article en
8 citations

Abstract

The integration of high-performance transparent top electrodes with the functional layers of transparent quantum dot light-emitting diodes (T-QLEDs) poses a notable challenge. This study presents a composite transparent top electrode composed of MXene and Ag NWs. The composite electrode demonstrates exceptional transparency (84.6% at 620 nm) and low sheet resistance (16.07 Ω sq<sup>-1</sup>), rendering it suitable for integration into T-QLEDs. The inclusion of MXene nanosheets in the composite electrode serves a dual role: adjusting the work function to enhance electron injection efficiency and enhancing the interface between Ag NWs and the emissive layer, thereby mitigating the common issue of interfacial resistance in conventional transparent electrodes. This strategic amalgamation results in notable improvements in device performance, yielding a maximum current efficiency of 23.12 cd A<sup>-1</sup>, an external quantum efficiency of 13.98%, and a brightness of 21,015 cd m<sup>-2</sup>. These performance metrics surpass those achieved by T-LEDs employing pristine Ag NW electrodes. This study offers valuable insights into T-QLED device advancement and provides a promising approach for transparent electrode fabrication in optoelectronic applications.

ACS Applied Materials & InterfacesVol. 16(40)
University of Macau (MO), Jiangmen Polytechnic (CN), Wuyi University (CN)
Department of Education of Guangdong Province, Basic and Applied Basic Research Foundation of Guangdong Province
Affordable and clean energy
Openalex Percentile: Top 23%
Quantum Dots Synthesis And Properties
0.94
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