Tilted-chiral-state-induced topological Hall effect in chiral magnetic soliton host Cr1/3TaS2

Chromium-intercalated Cr1/3TaS2 is well known for hosting a nontrivial chiral magnetic soliton lattice (CSL) with the reported highest Curie temperature (TC∼151 K) and strongest spin–orbit coupling, which has significant applications in gigahertz and high-speed spintronic devices. Herein, we thoroughly investigate the magneto-electrical transport properties of Cr1/3TaS2 single crystals. For H//ab, our magnetoresistance (MR) measurements reveal distinctive step-like behaviors, which are attributed to the formation and annihilation of chiral magnetic solitons. When under an oblique field, similar but weaker MR behaviors are observed compared to H//ab, indicating the appearance of an inclination-field-induced tilted-CSL. A topological Hall effect is observed under an oblique field, which is suggested to be induced by a nonzero topological charge density resulting from the tilted chiral states. The Cr1/3TaS2 offers an intriguing platform for studying the impact of chiral magnetic structures on magneto-electrical properties, which holds promise for both future spintronic device applications and fundamental investigation.

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Publication Details

Journal
Applied Physics Letters
Published
2024-09-23
DOI
https://doi.org/10.1063/5.0226822
Citations
1
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
0.34

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article

Tilted-chiral-state-induced topological Hall effect in chiral magnetic soliton host Cr1/3TaS2

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1 citations
Applied Physics Letters
Magnetic properties of thin films
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article

Tilted-chiral-state-induced topological Hall effect in chiral magnetic soliton host Cr1/3TaS2

Aina Wang, Wei Liu, Chunlan Ma, Min Ge, Jiyu Fan, Azizur Rahman, Yuyan Han, Zan Du, Wei Tong, Lei Zhang, Yuheng Zhang, Li Pi, Zhe Qu
article en
1 citations

Abstract

Chromium-intercalated Cr1/3TaS2 is well known for hosting a nontrivial chiral magnetic soliton lattice (CSL) with the reported highest Curie temperature (TC∼151 K) and strongest spin–orbit coupling, which has significant applications in gigahertz and high-speed spintronic devices. Herein, we thoroughly investigate the magneto-electrical transport properties of Cr1/3TaS2 single crystals. For H//ab, our magnetoresistance (MR) measurements reveal distinctive step-like behaviors, which are attributed to the formation and annihilation of chiral magnetic solitons. When under an oblique field, similar but weaker MR behaviors are observed compared to H//ab, indicating the appearance of an inclination-field-induced tilted-CSL. A topological Hall effect is observed under an oblique field, which is suggested to be induced by a nonzero topological charge density resulting from the tilted chiral states. The Cr1/3TaS2 offers an intriguing platform for studying the impact of chiral magnetic structures on magneto-electrical properties, which holds promise for both future spintronic device applications and fundamental investigation.

Applied Physics LettersVol. 125(13)
University of Science and Technology of China (CN), Anhui University (CN), Chinese Academy of Sciences (CN), Hefei Institutes of Physical Science (CN), Suzhou University of Science and Technology (CN), High Magnetic Field Laboratory (CN), Hefei National Center for Physical Sciences at Nanoscale (CN), Nanjing University of Aeronautics and Astronautics (CN)
National Natural Science Foundation of China, Alliance of International Science Organizations
Openalex Percentile: Top 40%
Magnetic properties of thin films
0.34
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