Topological phases driven by orbital entanglement in Transition Metal Oxide Perovskite interfaces

The deceptively simple crystallographic structure of early transition metal oxide perovskites belies the complexity and variety of electronic, magnetic and structural phases that they display. Structural defects, rotations, tilts, deformations of the oxygen-transition metal element octahedra help explain many of these phenomena. Another key player is the orbital degree of freedom of the d-ion. It may lead to a quantum entanglement of the materials electronic wavefunctions which promotes topological states in low dimensional geometries. In this report we present a study of select topological properties at surfaces or heterostructure interfaces of a subset of these perovskites when the orientation of the structure is along the (001) or (111) direction. In contrast to the extensively studied classes of topological insulators, topology in these systems is a characteristic property of the conducting regime, thus endowing the compounds with potential spintronic and quantum computing functionalities. We conclude this communication with a personal tribute to Gérard Toulouse (in French).

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Publication Details

Journal
Comptes Rendus Physique
Published
2024-09-19
DOI
https://doi.org/10.5802/crphys.190
Primary Topic
Electronic and Structural Properties of Oxides
Type
article
Field-Weighted Citation Impact
0.00

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article

Topological phases driven by orbital entanglement in Transition Metal Oxide Perovskite interfaces

M. Gabay
Comptes Rendus Physique
Electronic and Structural Properties of Oxides
article

Topological phases driven by orbital entanglement in Transition Metal Oxide Perovskite interfaces

M. Gabay
article en

Abstract

The deceptively simple crystallographic structure of early transition metal oxide perovskites belies the complexity and variety of electronic, magnetic and structural phases that they display. Structural defects, rotations, tilts, deformations of the oxygen-transition metal element octahedra help explain many of these phenomena. Another key player is the orbital degree of freedom of the d-ion. It may lead to a quantum entanglement of the materials electronic wavefunctions which promotes topological states in low dimensional geometries. In this report we present a study of select topological properties at surfaces or heterostructure interfaces of a subset of these perovskites when the orientation of the structure is along the (001) or (111) direction. In contrast to the extensively studied classes of topological insulators, topology in these systems is a characteristic property of the conducting regime, thus endowing the compounds with potential spintronic and quantum computing functionalities. We conclude this communication with a personal tribute to Gérard Toulouse (in French).

Comptes Rendus PhysiqueVol. 25(G1)
Laboratoire de physique des Solides (FR)
Université de Liège, Université de Genève, Université Paris-Saclay
Openalex Percentile: Top 90%
Electronic and Structural Properties of Oxides
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