Li-ion Battery Material phase prediction through Hierarchical Curriculum Learning

Li-ion Batteries (LIB), one of the most efficient energy storage devices, are widely adopted in many industrial applications. Imaging data of these battery electrodes obtained from X-ray tomography can explain the distribution of material constituents and allow reconstructions to study electron transport pathways. Therefore, it can eventually help quantify various associated properties of electrodes (e.g., volume-specific surface area, porosity) which determine the performance of batteries. However, these images often suffer from low image contrast between multiple material constituents , making it difficult for humans to distinguish and characterize these constituents through visualization. A minor error in detecting distributions among the material constituents can lead to a high error in the calculated parameters of material properties.We present a novel hierarchical curriculum learning framework to address the complex task of estimating material constituent distribution in battery electrodes. To provide spatially smooth prediction, our framework comprises three modules: (i) an uncertainty-aware model trained to yield inferences conditioned upon global knowledge of material distribution, (ii) a technique to capture relatively more fine-grained (local) distributional signals, (iii) an aggregator to appropriately fuse the local and global effects towards obtaining the final distribution.

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Publication Details

Journal
OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information)
Published
2024-09-04
Primary Topic
Machine Learning in Materials Science
Type
article

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article

Li-ion Battery Material phase prediction through Hierarchical Curriculum Learning

Anika Tabassum
OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information)
Machine Learning in Materials Science
article

Li-ion Battery Material phase prediction through Hierarchical Curriculum Learning

Anika Tabassum
article en

Abstract

Li-ion Batteries (LIB), one of the most efficient energy storage devices, are widely adopted in many industrial applications. Imaging data of these battery electrodes obtained from X-ray tomography can explain the distribution of material constituents and allow reconstructions to study electron transport pathways. Therefore, it can eventually help quantify various associated properties of electrodes (e.g., volume-specific surface area, porosity) which determine the performance of batteries. However, these images often suffer from low image contrast between multiple material constituents , making it difficult for humans to distinguish and characterize these constituents through visualization. A minor error in detecting distributions among the material constituents can lead to a high error in the calculated parameters of material properties.We present a novel hierarchical curriculum learning framework to address the complex task of estimating material constituent distribution in battery electrodes. To provide spatially smooth prediction, our framework comprises three modules: (i) an uncertainty-aware model trained to yield inferences conditioned upon global knowledge of material distribution, (ii) a technique to capture relatively more fine-grained (local) distributional signals, (iii) an aggregator to appropriately fuse the local and global effects towards obtaining the final distribution.

OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information)
U.S. Department of Energy, Office of Science, Office of Electricity, Advanced Scientific Computing Research, Oak Ridge National Laboratory
Quality Education
Machine Learning in Materials Science
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Li-ion Battery Material phase prediction through Hierarchical Curriculum Learning — Anika Tabassum · OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (2024) | TGRS Research Map | TGRS