Revealing hidden medium-range order in silicate glass formers using many-body correlation functions

The medium-range order in amorphous systems is believed to be related to quantities like dynamic heterogeneity, glass-formation ability, or the elastic properties of the glass. So far, however, there has been no simple way to characterize this order. Here, the authors use a novel many-body correlation function that allows to characterize this order. Applying this approach to sodium silicate glasses reveals that in these systems the temperature and compositional dependence of the medium-range order is surprisingly complex.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2024-09-17
DOI
https://doi.org/10.1103/physrevb.110.104203
Citations
9
Primary Topic
Glass properties and applications
Type
article
Field-Weighted Citation Impact
2.10

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article

Revealing hidden medium-range order in silicate glass formers using many-body correlation functions

Walter Kob, Zhen Zhang
9 citations
Physical review. B./Physical review. B
Glass properties and applications
2.10
article

Revealing hidden medium-range order in silicate glass formers using many-body correlation functions

Walter Kob, Zhen Zhang
article en
9 citations

Abstract

The medium-range order in amorphous systems is believed to be related to quantities like dynamic heterogeneity, glass-formation ability, or the elastic properties of the glass. So far, however, there has been no simple way to characterize this order. Here, the authors use a novel many-body correlation function that allows to characterize this order. Applying this approach to sodium silicate glasses reveals that in these systems the temperature and compositional dependence of the medium-range order is surprisingly complex.

Physical review. B./Physical review. BVol. 110(10)
Université de Montpellier (FR), Chengdu University of Technology (CN)
National Natural Science Foundation of China, Institut Universitaire de France
Climate action
Openalex Percentile: Top 14%
Glass properties and applications
2.10
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