Enhancing the performance of catalysts in turbulent premixed fuel-lean hydrogen/air combustion

• Turbulent catalytic combustion of premixed H 2 /air lean and ultra-lean mixtures. • Staggered cylinders enhance mass and heat convection, intensifying the catalytic process. • The non-planar reactor with half and full cylinders boosts H 2 conversion by 30.7 %. • Effective discrete coating reduces the amount of catalyst used by up to 50 %. Catalytic-aided combustion is a proven technique for burning highly lean and ultra-lean mixtures of hydrogen and air. However, the noble catalyst required for combustion is naturally scarce and therefore expensive. In this study, we focus on a numerical investigation to determine the best way of coating a platinum catalyst inside a catalytic hydrogen reactor. We study various planar and non-planar reactors and find that the reactor with a combination of half and full cylinders is the most effective in H 2 conversion. Compared to an equivalent catalytic planar reactor, the non-planar configuration increases the H 2 conversion by 30.7 %. The results show that enhancing mass and heat convection can significantly increase the H 2 conversion. Furthermore, in a non-planar reactor, surfaces with an enhanced mass and heat transfer can achieve up to 50 % catalyst savings when coated with a catalyst, while still maintaining a conversion rate of 2 kg/s per unit of catalytically-coated surface area.

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Publication Details

Journal
Chemical Engineering Science
Published
2024-09-17
DOI
https://doi.org/10.1016/j.ces.2024.120747
Citations
4
Primary Topic
Combustion and flame dynamics
Type
article
Field-Weighted Citation Impact
1.50

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article

Enhancing the performance of catalysts in turbulent premixed fuel-lean hydrogen/air combustion

S. David Jackson, Nader Karimi, Md Nur Alam Mondal, Manosh C. Paul
4 citations
Chemical Engineering Science
Combustion and flame dynamics
1.50
article

Enhancing the performance of catalysts in turbulent premixed fuel-lean hydrogen/air combustion

S. David Jackson, Nader Karimi, Md Nur Alam Mondal, Manosh C. Paul
article en
4 citations

Abstract

• Turbulent catalytic combustion of premixed H 2 /air lean and ultra-lean mixtures. • Staggered cylinders enhance mass and heat convection, intensifying the catalytic process. • The non-planar reactor with half and full cylinders boosts H 2 conversion by 30.7 %. • Effective discrete coating reduces the amount of catalyst used by up to 50 %. Catalytic-aided combustion is a proven technique for burning highly lean and ultra-lean mixtures of hydrogen and air. However, the noble catalyst required for combustion is naturally scarce and therefore expensive. In this study, we focus on a numerical investigation to determine the best way of coating a platinum catalyst inside a catalytic hydrogen reactor. We study various planar and non-planar reactors and find that the reactor with a combination of half and full cylinders is the most effective in H 2 conversion. Compared to an equivalent catalytic planar reactor, the non-planar configuration increases the H 2 conversion by 30.7 %. The results show that enhancing mass and heat convection can significantly increase the H 2 conversion. Furthermore, in a non-planar reactor, surfaces with an enhanced mass and heat transfer can achieve up to 50 % catalyst savings when coated with a catalyst, while still maintaining a conversion rate of 2 kg/s per unit of catalytically-coated surface area.

Chemical Engineering ScienceVol. 301
Queen Mary University of London (GB), University of Glasgow (GB)
Government of the United Kingdom, Commonwealth Scholarship Commission, Paul Scherrer Institut, China Scholarship Council, Engineering and Physical Sciences Research Council
Affordable and clean energy
Openalex Percentile: Top 20%
Combustion and flame dynamics
1.50
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