Long-Range Ballistic Propagation of 80% Excitonic Fraction Polaritons in a Perovskite Metasurface at Room Temperature

Exciton-polaritons, hybrid light-matter excitations arising from the strong coupling between excitons in semiconductors and photons in photonic nanostructures, are crucial for exploring the physics of quantum fluids of light and developing all-optical devices. Achieving room temperature propagation of polaritons with a large excitonic fraction is challenging but vital, e.g., for nonlinear light transport. We report on room temperature propagation of exciton-polaritons in a metasurface made from a subwavelength lattice of perovskite pillars. The large Rabi splitting, much greater than the optical phonon energy, decouples the lower polariton band from the phonon bath of the perovskite. These cooled polaritons, in combination with the high group velocity achieved through the metasurface design, enable long-range propagation, exceeding hundreds of micrometers even with an 80% excitonic component. Furthermore, the design of the metasurface introduces an original mechanism for unidirectional propagation through polarization control, suggesting a new avenue for the development of advanced polaritonic devices.

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Publication Details

Journal
Nano Letters
Published
2024-09-13
DOI
https://doi.org/10.1021/acs.nanolett.4c02696
Citations
7
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
2.36

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article

Long-Range Ballistic Propagation of 80% Excitonic Fraction Polaritons in a Perovskite Metasurface at Room Temperature

Dario Gerace, Simone Zanotti, Nguyen Ha My Dang, Hai Son Nguyen et al.
7 citations
Nano Letters
Strong Light-Matter Interactions
2.36
article

Long-Range Ballistic Propagation of 80% Excitonic Fraction Polaritons in a Perovskite Metasurface at Room Temperature

Dario Gerace, Simone Zanotti, Nguyen Ha My Dang, Hai Son Nguyen, Christian Seassal, Emmanuelle Deleporte, Emmanuel Drouard, Gaëlle Trippé-Allard, Céline Chevalier
article en
7 citations

Abstract

Exciton-polaritons, hybrid light-matter excitations arising from the strong coupling between excitons in semiconductors and photons in photonic nanostructures, are crucial for exploring the physics of quantum fluids of light and developing all-optical devices. Achieving room temperature propagation of polaritons with a large excitonic fraction is challenging but vital, e.g., for nonlinear light transport. We report on room temperature propagation of exciton-polaritons in a metasurface made from a subwavelength lattice of perovskite pillars. The large Rabi splitting, much greater than the optical phonon energy, decouples the lower polariton band from the phonon bath of the perovskite. These cooled polaritons, in combination with the high group velocity achieved through the metasurface design, enable long-range propagation, exceeding hundreds of micrometers even with an 80% excitonic component. Furthermore, the design of the metasurface introduces an original mechanism for unidirectional propagation through polarization control, suggesting a new avenue for the development of advanced polaritonic devices.

Nano LettersVol. 24(38)
Université Claude Bernard Lyon 1 (FR), École Centrale de Lyon (FR), Centre National de la Recherche Scientifique (FR), Institut Universitaire de France (FR), University of Pavia (IT), Université Paris-Saclay (FR), Institut des Nanotechnologies de Lyon (FR), CentraleSupélec (FR), Institut National des Sciences Appliquées de Lyon (FR), École d'Ingénieurs en Chimie et Sciences du Numérique (FR)
Agence Nationale de la Recherche, Ministero dell'Università e della Ricerca
Openalex Percentile: Top 11%
Strong Light-Matter Interactions
2.36
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