Correlation functions from tensor network influence functionals: The case of the spin-boson model

We investigate the application of matrix product state (MPS) representations of the influence functionals (IFs) for the calculation of real-time equilibrium correlation functions in open quantum systems. Focusing specifically on the unbiased spin-boson model, we explore the use of IF-MPSs for complex time propagation, as well as IF-MPSs for constructing correlation functions in the steady state. We examine three different IF approaches: one based on the Kadanoff-Baym contour targeting correlation functions at all times, one based on a complex contour targeting the correlation function at a single time, and a steady state formulation, which avoids imaginary or complex times, while providing access to correlation functions at all times. We show that within the IF language, the steady state formulation provides a powerful approach to evaluate equilibrium correlation functions.

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Publication Details

Journal
The Journal of Chemical Physics
Published
2024-09-13
DOI
https://doi.org/10.1063/5.0224880
Citations
8
Primary Topic
Spectroscopy and Quantum Chemical Studies
Type
article
Field-Weighted Citation Impact
2.70

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article

Correlation functions from tensor network influence functionals: The case of the spin-boson model

Nathan Ng, David R. Reichman, Gunhee Park, Lachlan P. Lindoy et al.
8 citations
The Journal of Chemical Physics
Spectroscopy and Quantum Chemical Studies
2.70
article

Correlation functions from tensor network influence functionals: The case of the spin-boson model

Nathan Ng, David R. Reichman, Gunhee Park, Lachlan P. Lindoy, Haimi Nguyen, Andrew J. Millis, Garnet Kin‐Lic Chan
article en
8 citations

Abstract

We investigate the application of matrix product state (MPS) representations of the influence functionals (IFs) for the calculation of real-time equilibrium correlation functions in open quantum systems. Focusing specifically on the unbiased spin-boson model, we explore the use of IF-MPSs for complex time propagation, as well as IF-MPSs for constructing correlation functions in the steady state. We examine three different IF approaches: one based on the Kadanoff-Baym contour targeting correlation functions at all times, one based on a complex contour targeting the correlation function at a single time, and a steady state formulation, which avoids imaginary or complex times, while providing access to correlation functions at all times. We show that within the IF language, the steady state formulation provides a powerful approach to evaluate equilibrium correlation functions.

The Journal of Chemical PhysicsVol. 161(10)
California Institute of Technology (US), National Physical Laboratory (GB), Flatiron Health (United States) (US), Columbia University (US)
U.S. Department of Energy, Engineering and Physical Sciences Research Council
Openalex Percentile: Top 9%
Spectroscopy and Quantum Chemical Studies
2.70
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Correlation functions from tensor network influence functionals: The case of the spin-boson model — Nathan Ng, David R. Reichman, et al. · The Journal of Chemical Physics (2024) | TGRS Research Map | TGRS