Correlation functions from tensor network influence functionals: The case of the spin-boson model
We investigate the application of matrix product state (MPS) representations of the influence functionals (IFs) for the calculation of real-time equilibrium correlation functions in open quantum systems. Focusing specifically on the unbiased spin-boson model, we explore the use of IF-MPSs for complex time propagation, as well as IF-MPSs for constructing correlation functions in the steady state. We examine three different IF approaches: one based on the Kadanoff-Baym contour targeting correlation functions at all times, one based on a complex contour targeting the correlation function at a single time, and a steady state formulation, which avoids imaginary or complex times, while providing access to correlation functions at all times. We show that within the IF language, the steady state formulation provides a powerful approach to evaluate equilibrium correlation functions.
Authors
- Nathan Ng (ORCID: https://orcid.org/0000-0002-0885-6036)
- David R. Reichman (ORCID: https://orcid.org/0000-0002-5265-5637)
- Gunhee Park (ORCID: https://orcid.org/0000-0002-2818-488X)
- Lachlan P. Lindoy (ORCID: https://orcid.org/0000-0002-1888-6490)
- Haimi Nguyen (ORCID: https://orcid.org/0000-0003-1685-445X)
- Andrew J. Millis (ORCID: https://orcid.org/0000-0001-9413-6344)
- Garnet Kin‐Lic Chan (ORCID: https://orcid.org/0000-0001-8009-6038)
Institutions
- California Institute of Technology (US)
- National Physical Laboratory (GB)
- Flatiron Health (United States) (US)
- Columbia University (US)
Publication Details
- Journal
- The Journal of Chemical Physics
- Published
- 2024-09-13
- DOI
- https://doi.org/10.1063/5.0224880
- Citations
- 8
- Primary Topic
- Spectroscopy and Quantum Chemical Studies
- Type
- article
- Field-Weighted Citation Impact
- 2.70
Funders
- U.S. Department of Energy
- Engineering and Physical Sciences Research Council