Monitoring CO <sub>2</sub> , CO and CH <sub>4</sub> , affected or not by ventilation and anthropogenic activities, in the galleries of the Underground Research Laboratory (URL) of Meuse/Haute-Marne

The alternation between periods of ventilation and non-ventilation of the galleries in the Meuse/Haute-Marne Underground Research Laboratory (URL) within the Callovian–Oxfordian argillaceous rock affects the contents of CO 2 , CO and CH 4 in atmospheric air. Monitoring the evolution of the gas composition in the galleries was conducted over a period of about 4 months. Two models of IR laser spectroscope (Picarro) were used, one to measure CO 2 , CO and CH 4 concentrations and the other to measure CH 4 isotopic compositions. The results show a night and day periodicity with the highest concentrations at night-time and the lowest during the daytime in the URL. Long-term monitoring of these gases at the surface shows the same evolution, but with different amplitudes. Moreover, in the URL, a weekday and weekend or holiday periodicity were superimposed. The concentrations of CO 2 in the galleries are influenced by human activities and ventilation. During working days, the galleries are ventilated, and human activities increase the CO 2 concentrations. Conversely, during weekends and holidays, CO 2 concentrations decrease owing to the cessation of ventilation and human activities, and consumption of CO 2 by concrete carbonation. The data analysis confirms a CH 4 source from the rock and reveals compelling evidence of CO sources that probably originate from rock and/or gallery engineered structure materials. Despite the difficulties in quantifying local sources and sinks of these gases, this study demonstrates the feasibility of obtaining valuable insights into their variability. This study provides information on potential sources and sinks of CO 2 , CO and CH 4 in this context.

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Publication Details

Journal
Journal of the Geological Society
Published
2024-09-10
DOI
https://doi.org/10.1144/jgs2023-149
Primary Topic
Air Quality Monitoring and Forecasting
Type
article
Field-Weighted Citation Impact
0.00

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article

Monitoring CO 2 , CO and CH 4 , affected or not by ventilation and anthropogenic activities, in the galleries of the Underground Research Laboratory (URL) of Meuse/Haute-Marne

Seny Keita, A. Vinsot, Mélanie Lundy, Guillaume Berthe et al.
Journal of the Geological Society
Air Quality Monitoring and Forecasting
article

Monitoring CO 2 , CO and CH 4 , affected or not by ventilation and anthropogenic activities, in the galleries of the Underground Research Laboratory (URL) of Meuse/Haute-Marne

Seny Keita, A. Vinsot, Mélanie Lundy, Guillaume Berthe, Bruno Garcia
article en

Abstract

The alternation between periods of ventilation and non-ventilation of the galleries in the Meuse/Haute-Marne Underground Research Laboratory (URL) within the Callovian–Oxfordian argillaceous rock affects the contents of CO 2 , CO and CH 4 in atmospheric air. Monitoring the evolution of the gas composition in the galleries was conducted over a period of about 4 months. Two models of IR laser spectroscope (Picarro) were used, one to measure CO 2 , CO and CH 4 concentrations and the other to measure CH 4 isotopic compositions. The results show a night and day periodicity with the highest concentrations at night-time and the lowest during the daytime in the URL. Long-term monitoring of these gases at the surface shows the same evolution, but with different amplitudes. Moreover, in the URL, a weekday and weekend or holiday periodicity were superimposed. The concentrations of CO 2 in the galleries are influenced by human activities and ventilation. During working days, the galleries are ventilated, and human activities increase the CO 2 concentrations. Conversely, during weekends and holidays, CO 2 concentrations decrease owing to the cessation of ventilation and human activities, and consumption of CO 2 by concrete carbonation. The data analysis confirms a CH 4 source from the rock and reveals compelling evidence of CO sources that probably originate from rock and/or gallery engineered structure materials. Despite the difficulties in quantifying local sources and sinks of these gases, this study demonstrates the feasibility of obtaining valuable insights into their variability. This study provides information on potential sources and sinks of CO 2 , CO and CH 4 in this context.

Journal of the Geological SocietyVol. 182(1)
IFP Énergies nouvelles (FR), Sorbonne Université (FR)
IFP Energies Nouvelles, Agence Nationale pour la Gestion des Déchets Radioactifs
Openalex Percentile: Top 86%
Air Quality Monitoring and Forecasting
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