Real- and reciprocal space characterization of the three-dimensional charge density wave in quasi-one-dimensional CuTe
Low-dimensional materials are susceptible to electronic instabilities such as charge density waves (CDWs), originating from a divergence in the Lindhard electron response function, combined with a finite electron-phonon coupling strength. In this paper, we present a detailed characterization of the CDW in the quasi-one-dimensional material CuTe, including (1) direct visualization of lattice distortion seen with noncontact atomic force microscopy in real space, (2) the out-of-plane momentum dependency of the CDW gap size of the quasi-one-dimensional bands by angle-resolved photoemission spectroscopy, and (3) coherent dynamics of a photoexcited phonon mode seen by time- and angle-resolved photoemission spectroscopy, with frequency and wave vector ${\mathit{q}}_{\text{CDW}}$ corresponding to the soft phonon modes predicted by theory. Furthermore, we find that the CDW gap closes through a transient band renormalization. We thus confirm that, despite the quasi-one-dimensional characteristics of CuTe, it hosts inherently three-dimensional CDWs.
Authors
- J. Hugo Dil (ORCID: https://orcid.org/0000-0002-6016-6120)
- Arnaud Magrez (ORCID: https://orcid.org/0000-0001-5933-7036)
- Michele Puppin (ORCID: https://orcid.org/0000-0002-1328-7165)
- Lukas Hellbrück (ORCID: https://orcid.org/0000-0002-9483-6612)
- Igor Sokolović (ORCID: https://orcid.org/0000-0003-1357-396X)
- Fei Guo (ORCID: https://orcid.org/0000-0002-3748-4016)
- Eduardo B. Guedes (ORCID: https://orcid.org/0000-0001-9638-0447)
Institutions
- TU Wien (AT)
- Paul Scherrer Institute (CH)
- École Polytechnique Fédérale de Lausanne (CH)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2024-09-09
- DOI
- https://doi.org/10.1103/physrevb.110.115112
- Citations
- 2
- Primary Topic
- Organic and Molecular Conductors Research
- Type
- article
- Field-Weighted Citation Impact
- 0.24
Funders
- Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung