High harmonic generation from electrons moving in topological spin textures

High harmonic generation (HHG) is a striking phenomenon, which reflects the ultrafast dynamics of electrons. Recently, it has been demonstrated that HHG can be used to reconstruct not only the energy band structure but also the geometric structure characterized by the Berry curvature. Here, we numerically investigate HHG arising from electrons coupled with a topological spin texture in a spin scalar chiral state where time reversal symmetry is broken. In this system, a sign change in scalar chirality alters the sign of the Berry curvature while keeping the energy band structure unchanged, allowing us to discuss purely geometrical effects on HHG. Notably, we found that, when the optical frequency is significantly lower than the energy gap, the sign of scalar chirality largely affects the longitudinal response parallel to the optical field rather than the transverse response. Our analysis suggests that this can be attributed to interband currents induced by the recombination of electron-hole pairs whose real-space trajectories are modulated by the anomalous velocity term.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2024-09-06
DOI
https://doi.org/10.1103/physrevb.110.125111
Citations
5
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
1.69

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article

High harmonic generation from electrons moving in topological spin textures

Yutaka Akagi, Shun Okumura, Shohei Imai, Atsushi Ono
5 citations
Physical review. B./Physical review. B
Laser-Matter Interactions and Applications
1.69
article

High harmonic generation from electrons moving in topological spin textures

Yutaka Akagi, Shun Okumura, Shohei Imai, Atsushi Ono
article en
5 citations

Abstract

High harmonic generation (HHG) is a striking phenomenon, which reflects the ultrafast dynamics of electrons. Recently, it has been demonstrated that HHG can be used to reconstruct not only the energy band structure but also the geometric structure characterized by the Berry curvature. Here, we numerically investigate HHG arising from electrons coupled with a topological spin texture in a spin scalar chiral state where time reversal symmetry is broken. In this system, a sign change in scalar chirality alters the sign of the Berry curvature while keeping the energy band structure unchanged, allowing us to discuss purely geometrical effects on HHG. Notably, we found that, when the optical frequency is significantly lower than the energy gap, the sign of scalar chirality largely affects the longitudinal response parallel to the optical field rather than the transverse response. Our analysis suggests that this can be attributed to interband currents induced by the recombination of electron-hole pairs whose real-space trajectories are modulated by the anomalous velocity term.

Physical review. B./Physical review. BVol. 110(12)
Tohoku University (JP), The University of Tokyo (JP)
Japan Society for the Promotion of Science, Japan Science and Technology Agency
Affordable and clean energy
Openalex Percentile: Top 16%
Laser-Matter Interactions and Applications
1.69
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