Kondo breakdown in multi-orbital Anderson lattices induced by destructive hybridization interference

In this paper we consider a multi-band extension to the periodic Anderson model. We use a single site DMFT(NRG) in order to study the impact of the conduction band mediated effective hopping of the correlated electrons between the correlated orbitals onto the heavy Fermi-liquid formation. Whereas the hybridization of a single impurity model with two distinct conduction bands always adds up constructively, T_{K}\propto \exp(-\mathrm{const}\, U/(\Gamma_1+\Gamma_2)) <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:msub> <mml:mi>T</mml:mi> <mml:mi>K</mml:mi> </mml:msub> <mml:mo>∝</mml:mo> <mml:mo>exp</mml:mo> <mml:mo stretchy="false" form="prefix">(</mml:mo> <mml:mo>−</mml:mo> <mml:mstyle mathvariant="normal"> <mml:mi>c</mml:mi> <mml:mi>o</mml:mi> <mml:mi>n</mml:mi> <mml:mi>s</mml:mi> <mml:mi>t</mml:mi> </mml:mstyle> <mml:mspace width="0.167em"/> <mml:mi>U</mml:mi> <mml:mi>/</mml:mi> <mml:mo stretchy="false" form="prefix">(</mml:mo> <mml:msub> <mml:mi>Γ</mml:mi> <mml:mn>1</mml:mn> </mml:msub> <mml:mo>+</mml:mo> <mml:msub> <mml:mi>Γ</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:mo stretchy="false" form="postfix">)</mml:mo> <mml:mo stretchy="false" form="postfix">)</mml:mo> </mml:mrow> </mml:math> , we show that this does not have to be the case in lattice models, where, in remarkable contrast, also an low-energy Fermi-liquid scale T_0\propto \exp(-\mathrm{const}\, U/(\Gamma_1-\Gamma_2)) <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:msub> <mml:mi>T</mml:mi> <mml:mn>0</mml:mn> </mml:msub> <mml:mo>∝</mml:mo> <mml:mo>exp</mml:mo> <mml:mo stretchy="false" form="prefix">(</mml:mo> <mml:mo>−</mml:mo> <mml:mstyle mathvariant="normal"> <mml:mi>c</mml:mi> <mml:mi>o</mml:mi> <mml:mi>n</mml:mi> <mml:mi>s</mml:mi> <mml:mi>t</mml:mi> </mml:mstyle> <mml:mspace width="0.167em"/> <mml:mi>U</mml:mi> <mml:mi>/</mml:mi> <mml:mo stretchy="false" form="prefix">(</mml:mo> <mml:msub> <mml:mi>Γ</mml:mi> <mml:mn>1</mml:mn> </mml:msub> <mml:mo>−</mml:mo> <mml:msub> <mml:mi>Γ</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:mo stretchy="false" form="postfix">)</mml:mo> <mml:mo stretchy="false" form="postfix">)</mml:mo> </mml:mrow> </mml:math> can emerge due to quantum interference effects in multi-band models, where U <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mi>U</mml:mi> </mml:math> denotes the local Coulomb matrix element of the correlated orbitals and \Gamma_i <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:msub> <mml:mi>Γ</mml:mi> <mml:mi>i</mml:mi> </mml:msub> </mml:math> the local hybridization strength of band i <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mi>i</mml:mi> </mml:math> . At high symmetry points, heavy Fermi-liquid formation is suppressed which is associated with a breakdown of the Kondo effect. This results in an asymptotically scale-invariant (i.e., power-law) spectrum of the correlated orbitals \propto|\omega|^{1/3} <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mo>∝</mml:mo> <mml:mo stretchy="false" form="prefix">|</mml:mo> <mml:mi>ω</mml:mi> <mml:msup> <mml:mo stretchy="false" form="prefix">|</mml:mo> <mml:mrow> <mml:mn>1</mml:mn> <mml:mi>/</mml:mi> <mml:mn>3</mml:mn> </mml:mrow> </mml:msup> </mml:mrow> </mml:math> , indicating non-Fermi liquid properties of the quantum critical point, and a small Fermi surface including only the light quasi-particles. This orbital selective Mott phase demonstrates the possibility of metallic local criticality within the general framework of ordinary single site DMFT.

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Journal
SciPost Physics
Published
2024-09-02
DOI
https://doi.org/10.21468/scipostphys.17.3.069
Citations
1
Primary Topic
Rare-earth and actinide compounds
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article
Field-Weighted Citation Impact
0.31

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article

Kondo breakdown in multi-orbital Anderson lattices induced by destructive hybridization interference

Fabian Eickhoff, Frithjof B. Anders
1 citations
SciPost Physics
Rare-earth and actinide compounds
0.31
article

Kondo breakdown in multi-orbital Anderson lattices induced by destructive hybridization interference

Fabian Eickhoff, Frithjof B. Anders
article en
1 citations

Abstract

In this paper we consider a multi-band extension to the periodic Anderson model. We use a single site DMFT(NRG) in order to study the impact of the conduction band mediated effective hopping of the correlated electrons between the correlated orbitals onto the heavy Fermi-liquid formation. Whereas the hybridization of a single impurity model with two distinct conduction bands always adds up constructively, T_{K}\propto \exp(-\mathrm{const}\, U/(\Gamma_1+\Gamma_2)) <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:msub> <mml:mi>T</mml:mi> <mml:mi>K</mml:mi> </mml:msub> <mml:mo>∝</mml:mo> <mml:mo>exp</mml:mo> <mml:mo stretchy="false" form="prefix">(</mml:mo> <mml:mo>−</mml:mo> <mml:mstyle mathvariant="normal"> <mml:mi>c</mml:mi> <mml:mi>o</mml:mi> <mml:mi>n</mml:mi> <mml:mi>s</mml:mi> <mml:mi>t</mml:mi> </mml:mstyle> <mml:mspace width="0.167em"/> <mml:mi>U</mml:mi> <mml:mi>/</mml:mi> <mml:mo stretchy="false" form="prefix">(</mml:mo> <mml:msub> <mml:mi>Γ</mml:mi> <mml:mn>1</mml:mn> </mml:msub> <mml:mo>+</mml:mo> <mml:msub> <mml:mi>Γ</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:mo stretchy="false" form="postfix">)</mml:mo> <mml:mo stretchy="false" form="postfix">)</mml:mo> </mml:mrow> </mml:math> , we show that this does not have to be the case in lattice models, where, in remarkable contrast, also an low-energy Fermi-liquid scale T_0\propto \exp(-\mathrm{const}\, U/(\Gamma_1-\Gamma_2)) <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:msub> <mml:mi>T</mml:mi> <mml:mn>0</mml:mn> </mml:msub> <mml:mo>∝</mml:mo> <mml:mo>exp</mml:mo> <mml:mo stretchy="false" form="prefix">(</mml:mo> <mml:mo>−</mml:mo> <mml:mstyle mathvariant="normal"> <mml:mi>c</mml:mi> <mml:mi>o</mml:mi> <mml:mi>n</mml:mi> <mml:mi>s</mml:mi> <mml:mi>t</mml:mi> </mml:mstyle> <mml:mspace width="0.167em"/> <mml:mi>U</mml:mi> <mml:mi>/</mml:mi> <mml:mo stretchy="false" form="prefix">(</mml:mo> <mml:msub> <mml:mi>Γ</mml:mi> <mml:mn>1</mml:mn> </mml:msub> <mml:mo>−</mml:mo> <mml:msub> <mml:mi>Γ</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:mo stretchy="false" form="postfix">)</mml:mo> <mml:mo stretchy="false" form="postfix">)</mml:mo> </mml:mrow> </mml:math> can emerge due to quantum interference effects in multi-band models, where U <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mi>U</mml:mi> </mml:math> denotes the local Coulomb matrix element of the correlated orbitals and \Gamma_i <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:msub> <mml:mi>Γ</mml:mi> <mml:mi>i</mml:mi> </mml:msub> </mml:math> the local hybridization strength of band i <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mi>i</mml:mi> </mml:math> . At high symmetry points, heavy Fermi-liquid formation is suppressed which is associated with a breakdown of the Kondo effect. This results in an asymptotically scale-invariant (i.e., power-law) spectrum of the correlated orbitals \propto|\omega|^{1/3} <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mo>∝</mml:mo> <mml:mo stretchy="false" form="prefix">|</mml:mo> <mml:mi>ω</mml:mi> <mml:msup> <mml:mo stretchy="false" form="prefix">|</mml:mo> <mml:mrow> <mml:mn>1</mml:mn> <mml:mi>/</mml:mi> <mml:mn>3</mml:mn> </mml:mrow> </mml:msup> </mml:mrow> </mml:math> , indicating non-Fermi liquid properties of the quantum critical point, and a small Fermi surface including only the light quasi-particles. This orbital selective Mott phase demonstrates the possibility of metallic local criticality within the general framework of ordinary single site DMFT.

SciPost PhysicsVol. 17(3)
TU Dortmund University (DE), Deutsches Zentrum für Luft- und Raumfahrt e. V. (DLR) (DE), Software (Germany) (DE)
Deutsche Forschungsgemeinschaft, Deutsches Zentrum für Luft- und Raumfahrt
Openalex Percentile: Top 44%
Rare-earth and actinide compounds
0.31
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