A ratiometric fluorescent electrospun film with high amine sensitivity and stability for visual monitoring of livestock meat freshness
Ratiometric fluorescent films with high amine sensitivity and stability were developed to monitor the freshness of beef and pork. Fluorescein isothiocyanate (FITC) and red carbon quantum dots (R-CQD) were used as the amine-responsive indicator and internal reference, respectively. The electrospun films prepared by immobilizing FITC and R-CQD complex (F-R) into polyvinylidene fluoride (PVDF) under 35 %, 55 % and 75 % of relative humidity (RH) were named F-R@PVDF-1, F-R@PVDF-2 and F-R@PVDF-3, respectively. In comparison, the F-R@PVDF-2 film exhibited the highest sensitivity to trimethylamine (TMA), demonstrating a limit of detection (<i>LOD</i>) value of 1.59 μM, and meanwhile high stability during storage with Δ<i>E</i> value of 1.99 after 14 days of storage at 4 °C. The F-R@PVDF-2 film also showed a significant fluorescent red-to-brown color change during meat freshness monitoring at 4 °C. Conclusively, this study reported a new ratiometric fluorescent film that can be used to track the freshness of meats in food packaging.
Authors
- Haroon Elrasheid Tahir (ORCID: https://orcid.org/0000-0003-3452-3857)
- Wenjun Song
- Xiaodong Zhai (ORCID: https://orcid.org/0000-0003-4906-7292)
- Fuyuan Ding
- Chenguang Zhou (ORCID: https://orcid.org/0000-0001-7844-8743)
- Xiaowei Huang (ORCID: https://orcid.org/0000-0001-9964-687X)
- Zhihua Li (ORCID: https://orcid.org/0000-0002-7709-5621)
- Xiaobo Zou (ORCID: https://orcid.org/0000-0001-5719-7025)
- Jiyong Shi (ORCID: https://orcid.org/0000-0002-8808-7256)
- Yue Sun (ORCID: https://orcid.org/0000-0001-7135-7427)
- Tingting Shen (ORCID: https://orcid.org/0000-0002-8446-9978)
- Yanxiao Li (ORCID: https://orcid.org/0000-0002-8171-0535)
- Yuhong Xue
- Di Zhang (ORCID: https://orcid.org/0000-0002-8531-0117)
- Xinai Zhang (ORCID: https://orcid.org/0000-0002-3901-0148)
Institutions
- Jiangsu University (CN)
Publication Details
- Journal
- Food Chemistry X
- Published
- 2024-09-02
- DOI
- https://doi.org/10.1016/j.fochx.2024.101801
- Citations
- 11
- Primary Topic
- Advanced biosensing and bioanalysis techniques
- Type
- article
- Field-Weighted Citation Impact
- 2.57
Funders
- National Natural Science Foundation of China
- Government of Jiangsu Province
- Natural Science Foundation of Jiangsu Province
- Agriculture Research System of China
- Priority Academic Program Development of Jiangsu Higher Education Institutions
- National Key Research and Development Program of China