Room temperature polariton spin switches based on Van der Waals superlattices

Transition-metal dichalcogenide monolayers possess large exciton binding energy and a robust valley degree of freedom, making them a viable platform for the development of spintronic devices capable of operating at room temperature. The development of such monolayer TMD-based spintronic devices requires strong spin-dependent interactions and effective spin transport. This can be achieved by employing exciton-polaritons. These hybrid light-matter states arising from the strong coupling of excitons and photons allow high-speed in-plane propagation and strong nonlinear interactions. Here, we demonstrate the operation of all-optical polariton spin switches by incorporating a WS<sub>2</sub> superlattice into a planar microcavity. We demonstrate spin-anisotropic polariton nonlinear interactions in a WS<sub>2</sub> superlattice at room temperature. As a proof-of-concept, we utilize these spin-dependent interactions to implement different spin switch geometries at ambient conditions, which show intrinsic sub-picosecond switching time and small footprint. Our findings offer new perspectives on manipulations of the polarization state in polaritonic systems and highlight the potential of atomically thin semiconductors for the development of next generation information processing devices.

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Publication Details

Journal
Nature Communications
Published
2024-09-01
DOI
https://doi.org/10.1038/s41467-024-51612-2
Citations
19
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
6.41

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article

Room temperature polariton spin switches based on Van der Waals superlattices

Qihua Xiong, Rui Su, D. Sanvitto, Antonio Fieramosca et al.
19 citations
Nature Communications
Strong Light-Matter Interactions
6.41
article

Room temperature polariton spin switches based on Van der Waals superlattices

Qihua Xiong, Rui Su, D. Sanvitto, Antonio Fieramosca, Ruiqi Bao, T. C. H. Liew, K. Dini, Jiaxin Zhao
article en
19 citations

Abstract

Transition-metal dichalcogenide monolayers possess large exciton binding energy and a robust valley degree of freedom, making them a viable platform for the development of spintronic devices capable of operating at room temperature. The development of such monolayer TMD-based spintronic devices requires strong spin-dependent interactions and effective spin transport. This can be achieved by employing exciton-polaritons. These hybrid light-matter states arising from the strong coupling of excitons and photons allow high-speed in-plane propagation and strong nonlinear interactions. Here, we demonstrate the operation of all-optical polariton spin switches by incorporating a WS<sub>2</sub> superlattice into a planar microcavity. We demonstrate spin-anisotropic polariton nonlinear interactions in a WS<sub>2</sub> superlattice at room temperature. As a proof-of-concept, we utilize these spin-dependent interactions to implement different spin switch geometries at ambient conditions, which show intrinsic sub-picosecond switching time and small footprint. Our findings offer new perspectives on manipulations of the polarization state in polaritonic systems and highlight the potential of atomically thin semiconductors for the development of next generation information processing devices.

Nature CommunicationsVol. 15(1)
Nanyang Technological University (SG), Istituto di Nanotecnologia (IT), Beijing Academy of Quantum Information Sciences (CN), Tsinghua University (CN)
Strong, Nanyang Technological University, National Natural Science Foundation of China, Tsinghua University, Ministry of Education, India, State Key Laboratory of Low-Dimensional Quantum Physics, National Key Research and Development Program of China
Affordable and clean energy
Openalex Percentile: Top 3%
Strong Light-Matter Interactions
6.41
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