Strong Spin-Motion Coupling in the Ultrafast Dynamics of Rydberg Atoms
Rydberg atoms in optical lattices and tweezers is now a well-established platform for simulating quantum spin systems. However, the role of the atoms' spatial wave function has not been examined in detail experimentally. Here, we show a strong spin-motion coupling emerging from the large variation of the interaction potential over the wave function spread. We observe its clear signature on the ultrafast many-body nanosecond-dynamics of atoms excited to a Rydberg S state, using picosecond pulses, from an unity-filling atomic Mott-insulator. We also propose an approach to tune arbitrarily the strength of the spin-motion coupling relative to the motional energy scale set by trapping potentials. Our work provides a new direction for exploring the dynamics of strongly correlated quantum systems by adding the motional degree of freedom to the Rydberg simulation toolbox.
Authors
- Takafumi Tomita (ORCID: https://orcid.org/0000-0003-2126-1392)
- Kenji Ohmori (ORCID: https://orcid.org/0000-0001-9584-5177)
- Miwako Mizoguchi
- T. P. Mahesh
- Seiji Sugawa (ORCID: https://orcid.org/0000-0002-2949-3617)
- Takuya Matsubara (ORCID: https://orcid.org/0000-0001-8869-7874)
- Vineet Bharti (ORCID: https://orcid.org/0000-0001-7927-3025)
- Sylvain de Léséleuc (ORCID: https://orcid.org/0000-0002-4761-5753)
- Masaya Kunimi (ORCID: https://orcid.org/0000-0002-2127-4807)
- Vikas Singh Chauhan (ORCID: https://orcid.org/0000-0002-4748-5960)
Institutions
- Tokyo University of Science (JP)
- National Institutes of Natural Sciences (JP)
- The Graduate University for Advanced Studies, SOKENDAI (JP)
- Institute for Molecular Science (JP)
- The University of Tokyo (JP)
Publication Details
- Journal
- Physical Review Letters
- Published
- 2024-08-30
- DOI
- https://doi.org/10.1103/physrevlett.133.093405
- Citations
- 14
- Primary Topic
- Cold Atom Physics and Bose-Einstein Condensates
- Type
- article
- Field-Weighted Citation Impact
- 4.73
Funders
- Ministry of Education, Culture, Sports, Science and Technology
- Japan Society for the Promotion of Science
- Moonshot Research and Development Program