Electron-phonon coupling and competing Kekulé orders in twisted bilayer graphene

Magic-angle twisted bilayer graphene has attracted significant attention for its strongly correlated phenomena. Recent scanning tunneling experiments have measured graphene-scale Kekul\'e charge ordering in some of the correlated insulators and nearby metallic phases. While most of these can be explained by the strain-induced incommensurate Kekul\'e spiral phase, the presence of Kekul\'e ordering in ultralow strain devices is unexpected within the existing theory. Using Hartree-Fock and strong-coupling calculations, the authors show that such observations can be rationalized by invoking electron-phonon coupling to zone-corner graphene phonons.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2024-08-29
DOI
https://doi.org/10.1103/physrevb.110.085160
Citations
22
Primary Topic
Graphene research and applications
Type
article
Field-Weighted Citation Impact
2.46

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article

Electron-phonon coupling and competing Kekulé orders in twisted bilayer graphene

Yves H. Kwan, S. A. Parameswaran, Nick Bultinck, Glenn Wagner et al.
22 citations
Physical review. B./Physical review. B
Graphene research and applications
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article

Electron-phonon coupling and competing Kekulé orders in twisted bilayer graphene

Yves H. Kwan, S. A. Parameswaran, Nick Bultinck, Glenn Wagner, Steven H. Simon, Erez Berg
article en
22 citations

Abstract

Magic-angle twisted bilayer graphene has attracted significant attention for its strongly correlated phenomena. Recent scanning tunneling experiments have measured graphene-scale Kekul\'e charge ordering in some of the correlated insulators and nearby metallic phases. While most of these can be explained by the strain-induced incommensurate Kekul\'e spiral phase, the presence of Kekul\'e ordering in ultralow strain devices is unexpected within the existing theory. Using Hartree-Fock and strong-coupling calculations, the authors show that such observations can be rationalized by invoking electron-phonon coupling to zone-corner graphene phonons.

Physical review. B./Physical review. BVol. 110(8)
Princeton University (US), University of Zurich (CH), Ghent University Hospital (BE), Ghent University (BE), Science Oxford (GB), Weizmann Institute of Science (IL)
Engineering and Physical Sciences Research Council, H2020 European Research Council
Openalex Percentile: Top 7%
Graphene research and applications
2.46
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Electron-phonon coupling and competing Kekulé orders in twisted bilayer graphene — Yves H. Kwan, S. A. Parameswaran, et al. · Physical review. B./Physical review. B (2024) | TGRS Research Map | TGRS