<i>In situ</i> generation and manipulation of mirror twin boundaries in transition metal dichalcogenides

The mirror twin boundary (MTB) within semiconducting transition metal dichalcogenides (TMDs) not only provides a versatile platform to explore exotic phenomena of one-dimensional (1D) systems, but also offers an effective building block to introduce novel electronic states in the TMDs. In spite of extensive efforts on introducing the MTBs in the TMDs, creating and manipulating the MTBs with custom-designed sites remains an outstanding challenge in experiment. Here we present a facile method for in situ generation of MTBs in three different TMDs at predetermined positions by scanning tunneling microscope (STM) tip pulses. In $\mathrm{MoT}{\mathrm{e}}_{2}$, the length and density of the MTBs can be further manipulated using a STM tip. Moreover, we demonstrate the ability to introduce uniform-sized and orderly arranged MTB triangular loops, which generate low-energy flat electronic bands in the $\mathrm{MoT}{\mathrm{e}}_{2}$. A periodic modulation in the density of states with a $3a$ period ($a$ is the lattice constant) is observed in the MTBs. Unexpectedly, our experiment indicates that the MTBs exhibit length preference with $3\mathit{Na}$ ($N$ is an integer), implying that the mechanism for the periodic modulation in the density of states also plays a role in affecting the formation of the MTBs.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2024-08-26
DOI
https://doi.org/10.1103/physrevb.110.l081407
Citations
4
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
0.47

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article

In situ generation and manipulation of mirror twin boundaries in transition metal dichalcogenides

Qi Zheng, Lin He, Mohan Zhang, Ya-Ning Ren et al.
4 citations
Physical review. B./Physical review. B
2D Materials and Applications
0.47
article

In situ generation and manipulation of mirror twin boundaries in transition metal dichalcogenides

Qi Zheng, Lin He, Mohan Zhang, Ya-Ning Ren, Chao Yan, Jiaqi He, Yaxin Zhao, Ruohan Zhang, Zihan Guo
article en
4 citations

Abstract

The mirror twin boundary (MTB) within semiconducting transition metal dichalcogenides (TMDs) not only provides a versatile platform to explore exotic phenomena of one-dimensional (1D) systems, but also offers an effective building block to introduce novel electronic states in the TMDs. In spite of extensive efforts on introducing the MTBs in the TMDs, creating and manipulating the MTBs with custom-designed sites remains an outstanding challenge in experiment. Here we present a facile method for in situ generation of MTBs in three different TMDs at predetermined positions by scanning tunneling microscope (STM) tip pulses. In $\mathrm{MoT}{\mathrm{e}}_{2}$, the length and density of the MTBs can be further manipulated using a STM tip. Moreover, we demonstrate the ability to introduce uniform-sized and orderly arranged MTB triangular loops, which generate low-energy flat electronic bands in the $\mathrm{MoT}{\mathrm{e}}_{2}$. A periodic modulation in the density of states with a $3a$ period ($a$ is the lattice constant) is observed in the MTBs. Unexpectedly, our experiment indicates that the MTBs exhibit length preference with $3\mathit{Na}$ ($N$ is an integer), implying that the mechanism for the periodic modulation in the density of states also plays a role in affecting the formation of the MTBs.

Physical review. B./Physical review. BVol. 110(8)
Ministry of Education of the People's Republic of China (CN), Hunan University (CN), Beijing Normal University (CN)
National Natural Science Foundation of China, China Postdoctoral Science Foundation, National Postdoctoral Program for Innovative Talents, National Key Research and Development Program of China, Fundamental Research Funds for the Central Universities
Openalex Percentile: Top 39%
2D Materials and Applications
0.47
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