Theory of topological exciton insulators and condensates in flat Chern bands

Excitons are the neutral quasiparticles that form when Coulomb interactions create bound states between electrons and holes. Due to their bosonic nature, excitons are expected to condense and exhibit superfluidity at sufficiently low temperatures. In interacting Chern insulators, excitons may inherit the nontrivial topology and quantum geometry from the underlying electron wavefunctions. We theoretically investigate the excitonic bound states and superfluidity in flat-band insulators pumped with light. We find that the exciton wavefunctions exhibit vortex structures in momentum space, with the total vorticity being equal to the difference of Chern numbers between the conduction and valence bands. Moreover, both the exciton binding energy and the exciton superfluid density are proportional to the Brillouin-zone average of the quantum metric and the Coulomb potential energy per unit cell. Spontaneous emission of circularly polarized light from radiative decay is a detectable signature of the exciton vorticity. We propose that the vorticity can also be experimentally measured via the nonlinear anomalous Hall effect, whereas the exciton superfluidity can be detected by voltage-drop quantization through a combination of quantum geometry and Aharonov-Casher effect. Topological excitons and their superfluid phase could be realized in flat bands of twisted Van der Waals heterostructures.

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Publication Details

Journal
Proceedings of the National Academy of Sciences
Published
2024-08-23
DOI
https://doi.org/10.1073/pnas.2401644121
Citations
20
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
6.75

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article

Theory of topological exciton insulators and condensates in flat Chern bands

Pouyan Ghaemi, Bruno Uchoa, Hong-Yi Xie, Matteo Mitrano
20 citations
Proceedings of the National Academy of Sciences
Topological Materials and Phenomena
6.75
article

Theory of topological exciton insulators and condensates in flat Chern bands

Pouyan Ghaemi, Bruno Uchoa, Hong-Yi Xie, Matteo Mitrano
article en
20 citations

Abstract

Excitons are the neutral quasiparticles that form when Coulomb interactions create bound states between electrons and holes. Due to their bosonic nature, excitons are expected to condense and exhibit superfluidity at sufficiently low temperatures. In interacting Chern insulators, excitons may inherit the nontrivial topology and quantum geometry from the underlying electron wavefunctions. We theoretically investigate the excitonic bound states and superfluidity in flat-band insulators pumped with light. We find that the exciton wavefunctions exhibit vortex structures in momentum space, with the total vorticity being equal to the difference of Chern numbers between the conduction and valence bands. Moreover, both the exciton binding energy and the exciton superfluid density are proportional to the Brillouin-zone average of the quantum metric and the Coulomb potential energy per unit cell. Spontaneous emission of circularly polarized light from radiative decay is a detectable signature of the exciton vorticity. We propose that the vorticity can also be experimentally measured via the nonlinear anomalous Hall effect, whereas the exciton superfluidity can be detected by voltage-drop quantization through a combination of quantum geometry and Aharonov-Casher effect. Topological excitons and their superfluid phase could be realized in flat bands of twisted Van der Waals heterostructures.

Proceedings of the National Academy of SciencesVol. 121(35)
The Graduate Center, CUNY (US), Harvard University (US), City University of New York (US), University of Oklahoma (US)
National Science Foundation, U.S. Department of Energy, Aspen Center for Physics, University of Oklahoma, Office of Science, Division of Materials Research, Basic Energy Sciences
Affordable and clean energy
Openalex Percentile: Top 2%
Topological Materials and Phenomena
6.75
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