Low-Temperature NO<sub>2</sub> Gas-Sensing System Based on Metal–Organic Framework-Derived In<sub>2</sub>O<sub>3</sub> Structures and Advanced Machine Learning Techniques

In the bustling metropolis of tomorrow, where pollution levels are a constant concern, a team of innovative researchers embarked on a quest to revolutionize air quality monitoring. In pursuit of this objective, this study embarked on the synthesis of indium oxide materials via a straightforward solvothermal method purposely for NO<sub>2</sub> detection. Through meticulous analysis of their gas-sensing capabilities, a remarkable discovery came to light. Among the materials tested, In<sub>2</sub>O<sub>3</sub> (IO-2) exhibited exceptional sensitivity toward 100 ppm of NO<sub>2</sub> gas at an optimal working temperature of 150 °C and even at room temperature (RT). The response value reached an impressive 12.69, showcasing the material's outstanding capability to detect NO<sub>2</sub> gas even at 100 ppb. Further investigation revealed a significant linear relationship (<i>R</i><sup>2</sup> = 0.89454) and commendable reproducibility, highlighting IO-2's potential as a reliable and stable sensing material. Moreover, machine learning techniques were utilized to predict the response characteristics of the sensing materials to various environmental conditions, concentrations of target gases, and operational parameters. This predictive capability can guide the design of more efficient and robust gas sensors, ultimately contributing to improved safety and environmental monitoring. As the demand for efficient, portable, and eco-friendly electronics continues to grow, these findings contribute to the development of sustainable and high-performance materials that can meet the needs of modern technology.

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Publication Details

Journal
Inorganic Chemistry
Published
2024-08-22
DOI
https://doi.org/10.1021/acs.inorgchem.4c02453
Citations
17
Primary Topic
Gas Sensing Nanomaterials and Sensors
Type
article
Field-Weighted Citation Impact
3.55

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article

Low-Temperature NO2 Gas-Sensing System Based on Metal–Organic Framework-Derived In2O3 Structures and Advanced Machine Learning Techniques

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17 citations
Inorganic Chemistry
Gas Sensing Nanomaterials and Sensors
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article

Low-Temperature NO2 Gas-Sensing System Based on Metal–Organic Framework-Derived In2O3 Structures and Advanced Machine Learning Techniques

Jesse Nii Okai Amu‐Darko, Guanjun Qiao, Enock Adjei Agyekum, Guiwu Liu, Sufaid Shah, Kareem Yusuf, Shahid Hussain, Rajesh Kumar Manavalan, Amensisa Negasa Begi
article en
17 citations

Abstract

In the bustling metropolis of tomorrow, where pollution levels are a constant concern, a team of innovative researchers embarked on a quest to revolutionize air quality monitoring. In pursuit of this objective, this study embarked on the synthesis of indium oxide materials via a straightforward solvothermal method purposely for NO<sub>2</sub> detection. Through meticulous analysis of their gas-sensing capabilities, a remarkable discovery came to light. Among the materials tested, In<sub>2</sub>O<sub>3</sub> (IO-2) exhibited exceptional sensitivity toward 100 ppm of NO<sub>2</sub> gas at an optimal working temperature of 150 °C and even at room temperature (RT). The response value reached an impressive 12.69, showcasing the material's outstanding capability to detect NO<sub>2</sub> gas even at 100 ppb. Further investigation revealed a significant linear relationship (<i>R</i><sup>2</sup> = 0.89454) and commendable reproducibility, highlighting IO-2's potential as a reliable and stable sensing material. Moreover, machine learning techniques were utilized to predict the response characteristics of the sensing materials to various environmental conditions, concentrations of target gases, and operational parameters. This predictive capability can guide the design of more efficient and robust gas sensors, ultimately contributing to improved safety and environmental monitoring. As the demand for efficient, portable, and eco-friendly electronics continues to grow, these findings contribute to the development of sustainable and high-performance materials that can meet the needs of modern technology.

Inorganic ChemistryVol. 63(35)
Jiangsu University (CN), Ural Federal University (RU), University of Sargodha (PK), King Saud University (SA), Affiliated Hospital of Jiangsu University (CN)
National Natural Science Foundation of China, King Saud University, Ministry of Science and Higher Education of the Russian Federation, Qinglan Project of Jiangsu Province of China, National Key Research and Development Program of China
Openalex Percentile: Top 7%
Gas Sensing Nanomaterials and Sensors
3.55
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