Real‐Space Imaging of Intrinsic Symmetry‐Breaking Spin Textures in a Kagome Lattice
The electronic orders in kagome materials have emerged as a fertile platform for studying exotic quantum states, and their intertwining with the unique kagome lattice geometry remains elusive. While various unconventional charge orders with broken symmetry is observed, the influence of kagome symmetry on magnetic order has so far not been directly observed. Here, using a high-resolution magnetic force microscopy, it is, for the first time, observed a new lattice form of noncollinear spin textures in the kagome ferromagnet in zero magnetic field. Under the influence of the sixfold rotational symmetry of the kagome lattice, the spin textures are hexagonal in shape and can further form a honeycomb lattice structure. Subsequent thermal cycling measurements reveal that these spin textures transform into a non-uniform in-plane ferromagnetic ground state at low temperatures and can fully rebuild at elevated temperatures, showing a strong second-order phase transition feature. Moreover, some out-of-plane magnetic moments persist at low temperatures, supporting the Kane-Mele scenario in explaining the emergence of the Dirac gap. The observations establish that the electronic properties, including both charge and spin orders, are strongly coupled with the kagome lattices.
Authors
- Wenjie Meng (ORCID: https://orcid.org/0000-0002-0446-1205)
- Yongcheng Deng (ORCID: https://orcid.org/0000-0003-4047-5388)
- Yuyan Han (ORCID: https://orcid.org/0000-0002-6704-8768)
- Qiyuan Feng (ORCID: https://orcid.org/0000-0002-4339-8237)
- Qingyou Lu (ORCID: https://orcid.org/0000-0003-1934-8165)
- Jihao Wang (ORCID: https://orcid.org/0000-0001-8920-1199)
- Mangyuan Ma (ORCID: https://orcid.org/0000-0003-3079-5564)
- Yimin Xiong (ORCID: https://orcid.org/0000-0003-2736-8334)
- Fusheng Ma (ORCID: https://orcid.org/0000-0002-2290-8744)
- Dong Zhang (ORCID: https://orcid.org/0000-0002-4227-665X)
- Yubin Hou
- Junbo Li (ORCID: https://orcid.org/0000-0002-1566-0306)
- Wei Tong (ORCID: https://orcid.org/0000-0002-1269-9512)
- Caihong Xie
Institutions
- University of Science and Technology of China (CN)
- Anhui University (CN)
- Nanjing Normal University (CN)
- Chinese Academy of Sciences (CN)
- Hefei Institutes of Physical Science (CN)
- Hefei University (CN)
- High Magnetic Field Laboratory (CN)
- Institute of Semiconductors (CN)
Publication Details
- Journal
- Advanced Science
- Published
- 2024-08-19
- DOI
- https://doi.org/10.1002/advs.202404088
- Citations
- 6
- Primary Topic
- Advanced Condensed Matter Physics
- Type
- article
- Field-Weighted Citation Impact
- 1.87
Funders
- National Natural Science Foundation of China
- Chinese Academy of Sciences
- National Key Research and Development Program of China