Neural Network Based Aliasing Spectral Decoupling Algorithm for Precise Mid-Infrared Multicomponent Gases Sensing

Owing to the overlapping and cross-interference of absorption lines in multicomponent gases, the simultaneous measurement of such gases via laser absorption spectroscopy frequently necessitates the use of supplementary pressure sensors to distinguish the spectral lines. Alternatively, it requires multiple lasers combined with time-division multiplexing to independently scan the absorption peaks of each gas, thereby preventing interference from other gases. This inevitably escalates both the cost of the system and the complexity of the gas pathway. In response to these challenges, a mid-infrared sensor employing a neural network-based decoupling algorithm for aliasing spectral is developed, enabling the simultaneous detection of methane(CH<sub>4</sub>), water vapor(H<sub>2</sub>O), and ethane(C<sub>2</sub>H<sub>6</sub>). The sensor system underwent evaluation in a controlled laboratory environment. Allan deviation analysis revealed that the minimum detection limits for CH<sub>4</sub>,H<sub>2</sub>O, and C<sub>2</sub>H<sub>6</sub> were 6.04, 118.44, and 1 ppb, respectively, with an averaging time of 3 s. The performance of the proposed sensor demonstrates that the aliasing spectral decoupling algorithm based on neural network combined with wavelength-modulated spectroscopy technology has the advantages of high sensitivity, low cost and low complexity, showing its potential for simultaneous detection of multicomponent trace gases in various fields.

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Publication Details

Journal
ACS Sensors
Published
2024-08-16
DOI
https://doi.org/10.1021/acssensors.4c01514
Citations
16
Primary Topic
Spectroscopy and Laser Applications
Type
article
Field-Weighted Citation Impact
3.85

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article

Neural Network Based Aliasing Spectral Decoupling Algorithm for Precise Mid-Infrared Multicomponent Gases Sensing

Yuan Cao, Guishi Wang, Kun Liu, Ligang Shao et al.
16 citations
ACS Sensors
Spectroscopy and Laser Applications
3.85
article

Neural Network Based Aliasing Spectral Decoupling Algorithm for Precise Mid-Infrared Multicomponent Gases Sensing

Yuan Cao, Guishi Wang, Kun Liu, Ligang Shao, Ruifeng Wang, Xiaoming Gao, Hao Xiong, Jiaoxu Mei
article en
16 citations

Abstract

Owing to the overlapping and cross-interference of absorption lines in multicomponent gases, the simultaneous measurement of such gases via laser absorption spectroscopy frequently necessitates the use of supplementary pressure sensors to distinguish the spectral lines. Alternatively, it requires multiple lasers combined with time-division multiplexing to independently scan the absorption peaks of each gas, thereby preventing interference from other gases. This inevitably escalates both the cost of the system and the complexity of the gas pathway. In response to these challenges, a mid-infrared sensor employing a neural network-based decoupling algorithm for aliasing spectral is developed, enabling the simultaneous detection of methane(CH<sub>4</sub>), water vapor(H<sub>2</sub>O), and ethane(C<sub>2</sub>H<sub>6</sub>). The sensor system underwent evaluation in a controlled laboratory environment. Allan deviation analysis revealed that the minimum detection limits for CH<sub>4</sub>,H<sub>2</sub>O, and C<sub>2</sub>H<sub>6</sub> were 6.04, 118.44, and 1 ppb, respectively, with an averaging time of 3 s. The performance of the proposed sensor demonstrates that the aliasing spectral decoupling algorithm based on neural network combined with wavelength-modulated spectroscopy technology has the advantages of high sensitivity, low cost and low complexity, showing its potential for simultaneous detection of multicomponent trace gases in various fields.

ACS SensorsVol. 9(9)
University of Science and Technology of China (CN), Chinese Academy of Sciences (CN), Hefei Institutes of Physical Science (CN)
National Natural Science Foundation of China, National Key Research and Development Program of China
Affordable and clean energy
Openalex Percentile: Top 5%
Spectroscopy and Laser Applications
3.85
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