Unconventional Thermophotonic Charge Density Wave

Charge-order states of broken symmetry, such as charge density wave (CDW), are able to induce exceptional physical properties, however, the precise understanding of the underlying physics is still elusive. Here, we combine fluctuational electrodynamics and density functional theory to reveal an unconventional thermophotonic effect in CDW-bearing TiSe_{2}, referred to as thermophotonic-CDW (tp-CDW). The interplay of plasmon polariton and CDW electron excitations give rise to an anomalous negative temperature dependency in thermal photons transport, offering an intuitive fingerprint for a transformation of the electron order. Additionally, the demonstrated nontrivial features of tp-CDW transition hold promise for a controllable manipulation of heat flow, which could be extensively utilized in various fields such as thermal science and electron dynamics, as well as in next-generation energy devices.

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Publication Details

Journal
Physical Review Letters
Published
2024-08-05
DOI
https://doi.org/10.1103/physrevlett.133.066902
Citations
12
Primary Topic
Thermal Radiation and Cooling Technologies
Type
article
Field-Weighted Citation Impact
3.13

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Unconventional Thermophotonic Charge Density Wave

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article

Unconventional Thermophotonic Charge Density Wave

Cheng-Long Zhou, Shuihua Yang, Mauro Antezza, Dino Novko, Cheng‐Wei Qiu, Yong Zhang, Zahra Torbatian, Hong-Liang Yi
article en
12 citations

Abstract

Charge-order states of broken symmetry, such as charge density wave (CDW), are able to induce exceptional physical properties, however, the precise understanding of the underlying physics is still elusive. Here, we combine fluctuational electrodynamics and density functional theory to reveal an unconventional thermophotonic effect in CDW-bearing TiSe_{2}, referred to as thermophotonic-CDW (tp-CDW). The interplay of plasmon polariton and CDW electron excitations give rise to an anomalous negative temperature dependency in thermal photons transport, offering an intuitive fingerprint for a transformation of the electron order. Additionally, the demonstrated nontrivial features of tp-CDW transition hold promise for a controllable manipulation of heat flow, which could be extensively utilized in various fields such as thermal science and electron dynamics, as well as in next-generation energy devices.

Physical Review LettersVol. 133(6)
National University of Singapore (SG), Institut Universitaire de France (FR), Harbin Institute of Technology (CN), Laboratoire Charles Coulomb (FR), Institute of Physics (HR), Institute for Research in Fundamental Sciences (IR), Donostia International Physics Center (ES)
National Research Foundation, National Research Foundation Singapore, Ministry of Education - Singapore, Agence Nationale de la Recherche, National Natural Science Foundation of China, Research Grants Council, University Grants Committee, Hrvatska Zaklada za Znanost, China Scholarship Council, Hong Kong University of Science and Technology
Affordable and clean energy
Openalex Percentile: Top 9%
Thermal Radiation and Cooling Technologies
3.13
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