Vertically Grown Bioinspired Diphenylalanine Nanowire-Coated Fabric for Oil–Water Separation

Due to the pervasive use of oil for energy and other industrial applications, solutions to oil-water separation have received a great deal of attention lately to address the environmental damage of oil spills and groundwater contamination. However, many of these separation methods are materially expensive and environmentally hazardous, require elaborate fabrication, or rely on large amounts of energy to function. Herein, we provide an effective low-cost method for oil-water separation based on the hydrophobicity induced by self-assembled bioinspired diphenylalanine peptide nanowires grown on polyester fabric. This modified polyester fabric mesh exhibits parahydrophobicity and oleophilicity due to the hierarchical nano-to-microscale surface roughness. This mesh also achieves consistent high water separation efficiencies of over 99% and an ultrahigh oil flux of up to 26.7 ± 5 kLm^-2·h^-1. The growth of bioinspired peptide-based nanostructures on fabrics using facile technique and their application in oil-water separation presents the potential for using bioinspired materials for environmental remediation while minimizing environmental footprint.