Quantum Efficiency and Vertical Position of Quantum Emitters in hBN Determined by Purcell Effect in Hybrid Metal-Dielectric Planar Photonic Structures

Color centers in hexagonal boron nitride (hBN) advantageously combine excellent photophysical properties with the potential for integration in highly compact devices. Progress toward scalable integration necessitates a high quantum efficiency and an efficient photon collection. In this context, we compare the optical characteristics of individual hBN color centers generated by electron irradiation in two different electromagnetic environments. We keep track of well-identified emitters that we characterize before and after the dry transfer of exfoliated crystals. This comparison provides information about their quantum efficiency, which we find close to unity, as well as their vertical position in the crystal with nanometric precision, which we find away from the flake surfaces. Our work suggests hybrid dielectric-metal planar structures as an efficient tool for characterizing quantum emitters in addition to improving the count rate and can be generalized to other emitters in 2D materials or in planar photonic structures.

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Publication Details

Journal
ACS Photonics
Published
2024-12-06
DOI
https://doi.org/10.1021/acsphotonics.4c01416
Citations
10
Primary Topic
Diamond and Carbon-based Materials Research
Type
article
Field-Weighted Citation Impact
1.17

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article

Quantum Efficiency and Vertical Position of Quantum Emitters in hBN Determined by Purcell Effect in Hybrid Metal-Dielectric Planar Photonic Structures

Aymeric Delteil, Aurélie Pierret, Domitille Gérard, Jean‐Pierre Hermier et al.
10 citations
ACS Photonics
Diamond and Carbon-based Materials Research
1.17
article

Quantum Efficiency and Vertical Position of Quantum Emitters in hBN Determined by Purcell Effect in Hybrid Metal-Dielectric Planar Photonic Structures

Aymeric Delteil, Aurélie Pierret, Domitille Gérard, Jean‐Pierre Hermier, Stéphanie Buil, Bruno Bérini, Helmi Fartas
article en
10 citations

Abstract

Color centers in hexagonal boron nitride (hBN) advantageously combine excellent photophysical properties with the potential for integration in highly compact devices. Progress toward scalable integration necessitates a high quantum efficiency and an efficient photon collection. In this context, we compare the optical characteristics of individual hBN color centers generated by electron irradiation in two different electromagnetic environments. We keep track of well-identified emitters that we characterize before and after the dry transfer of exfoliated crystals. This comparison provides information about their quantum efficiency, which we find close to unity, as well as their vertical position in the crystal with nanometric precision, which we find away from the flake surfaces. Our work suggests hybrid dielectric-metal planar structures as an efficient tool for characterizing quantum emitters in addition to improving the count rate and can be generalized to other emitters in 2D materials or in planar photonic structures.

ACS PhotonicsVol. 11(12)
Centre National de la Recherche Scientifique (FR), Université de Versailles Saint-Quentin-en-Yvelines (FR), Université Paris Cité (FR), Université Paris Sciences et Lettres (FR), Université Paris-Saclay (FR), École Normale Supérieure - PSL (FR), Sorbonne Université (FR), Sorbonne Paris Cité (FR), Groupe d’Étude de la Matière Condensée (FR)
Agence Nationale de la Recherche
Affordable and clean energy
Openalex Percentile: Top 19%
Diamond and Carbon-based Materials Research
1.17
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