Incommensurate charge-stripe correlations in the kagome superconductor CsV<sub>3</sub>Sb<sub>5–x</sub>Sn<sub>x</sub>

The class of AV<sub>3</sub>Sb<sub>5</sub> (A=K, Rb, Cs) kagome metals hosts unconventional charge density wave states seemingly intertwined with their low temperature superconducting phases. The nature of the coupling between these two states and the potential presence of nearby, competing charge instabilities however remain open questions. This phenomenology is strikingly highlighted by the formation of two ‘domes’ in the superconducting transition temperature upon hole-doping CsV<sub>3</sub>Sb<sub>5</sub>. Here we track the evolution of charge correlations upon the suppression of long-range charge density wave order in the first dome and into the second of the hole-doped kagome superconductor CsV<sub>3</sub>Sb<sub>5–x</sub>Sn<sub>x</sub>. Initially, hole-doping drives interlayer charge correlations to become short-ranged with their periodicity diminished along the interlayer direction. Beyond the peak of the first superconducting dome, the parent charge density wave state vanishes and incommensurate, quasi-1D charge correlations are stabilized in its place. These competing, unidirectional charge correlations demonstrate an inherent electronic rotational symmetry breaking in CsV<sub>3</sub>Sb<sub>5</sub>, and reveal a complex landscape of charge correlations within its electronic phase diagram. Our data suggest an inherent 2k<sub>ƒ</sub> charge instability and competing charge orders in the AV<sub>3</sub>Sb<sub>5</sub> class of kagome superconductors.

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Publication Details

Journal
OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information)
Published
2024-09-17
DOI
https://doi.org/10.1038/s41535-023-00570-x
Citations
44
Primary Topic
Topological Materials and Phenomena
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article

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article

Incommensurate charge-stripe correlations in the kagome superconductor CsV3Sb5–xSnx

Linus Kautzsch
44 citations
OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information)
Topological Materials and Phenomena
article

Incommensurate charge-stripe correlations in the kagome superconductor CsV3Sb5–xSnx

Linus Kautzsch
article en
44 citations

Abstract

The class of AV<sub>3</sub>Sb<sub>5</sub> (A=K, Rb, Cs) kagome metals hosts unconventional charge density wave states seemingly intertwined with their low temperature superconducting phases. The nature of the coupling between these two states and the potential presence of nearby, competing charge instabilities however remain open questions. This phenomenology is strikingly highlighted by the formation of two ‘domes’ in the superconducting transition temperature upon hole-doping CsV<sub>3</sub>Sb<sub>5</sub>. Here we track the evolution of charge correlations upon the suppression of long-range charge density wave order in the first dome and into the second of the hole-doped kagome superconductor CsV<sub>3</sub>Sb<sub>5–x</sub>Sn<sub>x</sub>. Initially, hole-doping drives interlayer charge correlations to become short-ranged with their periodicity diminished along the interlayer direction. Beyond the peak of the first superconducting dome, the parent charge density wave state vanishes and incommensurate, quasi-1D charge correlations are stabilized in its place. These competing, unidirectional charge correlations demonstrate an inherent electronic rotational symmetry breaking in CsV<sub>3</sub>Sb<sub>5</sub>, and reveal a complex landscape of charge correlations within its electronic phase diagram. Our data suggest an inherent 2k<sub>ƒ</sub> charge instability and competing charge orders in the AV<sub>3</sub>Sb<sub>5</sub> class of kagome superconductors.

OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information)
University of California, Santa Barbara (US)
National Science Foundation, U.S. Department of Energy, Research Corporation for Science Advancement, University of California, Santa Barbara, Division of Materials Research, Basic Energy Sciences
Topological Materials and Phenomena
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